en Research Paper Research Paper <span style="font-size:11pt"><span style="line-height:200%"><span style="font-family:Calibri,sans-serif"><span new="" roman="" style="font-family:" times="">The effect of different Nd and PT compositions on the electrical and ferroelectric properties of (1-y)Bi_1-xNd_xFeO₃-yPbTiO₃ solid solutions, where x = 0.05, 0.10, 0.15, 0.20 and y = 0.1, 0.2, 0.3, and 0.4, was investigated to optimise material performance. Nd doping enhances the frequency-dependent dielectric properties of produced solid solutions. However, an anomaly in the dielectric loss tangent, which is consistent with the Debye relaxation process, is observed for compositions with x˂0.10 and y&ge;0.2 values in the frequency range of 1 KHz to 1 MHz. Dielectric anomalies were more noticeable around the transition temperature in temperature-dependent dielectric characteristics plots, suggesting stronger magnetoelectric interactions. The decrease in the dielectric constant for solid solution compositions with y &ge;0.3 indicates the presence of MPB with BFO due to an increase in the tetragonal phase of the PbTiO3 compound. As Nd content increases, temperature-dependent dielectric permittivity predicts relaxor-type ferroelectric performance for y=0.4 composition of solid solutions. A ferroelectric investigation showed that saturation polarisation, remnant polarisation, and coercive field of all prepared solid solutions decrease with increased Nd doping. However, for y˃0.3 composition, a substantial rise in these parameters was observed, which is a result of electric order dominating over magnetic order in solid solutions. The study reveals that Nd doping reduces leakage current, making it a promising contender for future applications</span></span></span></span><br> &nbsp; Solid solution,Nd doping,Electrical,Ferroelectric,remnant polarization 1 10 http://ijmse.iust.ac.ir/browse.php?a_code=A-10-5042-2&slc_lang=en&sid=1 Ram Chhavi Sharma rcsharma@sgtuniversity.org 1800319475328460019575 1800319475328460019575 Yes Department of Physics, Faculty of Applied and Basic Sciences, SGT University Gurugram-122505, Haryana, India.